Valley dynamics of excitons in monolayer dichalcogenides

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Gerd Plechinger - , University of Regensburg (Author)
  • Philipp Nagler - , University of Regensburg (Author)
  • Ashish Arora - , University of Münster (Author)
  • Robert Schmidt - , University of Münster (Author)
  • Alexey Chernikov - , University of Regensburg (Author)
  • John Lupton - , University of Regensburg (Author)
  • Rudolf Bratschitsch - , University of Münster (Author)
  • Christian Schüller - , University of Regensburg (Author)
  • Tobias Korn - , University of Regensburg (Author)

Abstract

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these semiconducting materials, optically excited electron–hole pairs form tightly Coulomb-bound excitons with large binding energies. The selection rules for excitonic transitions allow for direct optical generation of a valley-polarized exciton population using resonant excitation. Here, we investigate the exciton valley dynamics in monolayers of three different TMDCs by means of time-resolved Kerr rotation at low temperatures. We observe pronounced differences in the valley dynamics of tungsten- and molybdenum-based TMDCs, which are directly related to the opposite order of the conduction-band spin splitting in these materials.

Details

Original languageEnglish
Article number1700131
JournalPhysica Status Solidi - Rapid Research Letters
Volume11
Issue number7
Publication statusPublished - Jul 2017
Peer-reviewedYes
Externally publishedYes

Keywords

Keywords

  • excitons, transition metal dichalcogenides, two-dimensional materials, valley dynamics, valleytronics