Valley dynamics of excitons in monolayer dichalcogenides
Research output: Contribution to journal › Research article › Contributed › peer-review
Contributors
Abstract
Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these semiconducting materials, optically excited electron–hole pairs form tightly Coulomb-bound excitons with large binding energies. The selection rules for excitonic transitions allow for direct optical generation of a valley-polarized exciton population using resonant excitation. Here, we investigate the exciton valley dynamics in monolayers of three different TMDCs by means of time-resolved Kerr rotation at low temperatures. We observe pronounced differences in the valley dynamics of tungsten- and molybdenum-based TMDCs, which are directly related to the opposite order of the conduction-band spin splitting in these materials.
Details
| Original language | English |
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| Article number | 1700131 |
| Journal | Physica Status Solidi - Rapid Research Letters |
| Volume | 11 |
| Issue number | 7 |
| Publication status | Published - Jul 2017 |
| Peer-reviewed | Yes |
| Externally published | Yes |
External IDs
| ORCID | /0000-0002-9213-2777/work/196666228 |
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Keywords
ASJC Scopus subject areas
Keywords
- excitons, transition metal dichalcogenides, two-dimensional materials, valley dynamics, valleytronics