Valley dynamics of excitons in monolayer dichalcogenides

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Gerd Plechinger - , Universität Regensburg (Autor:in)
  • Philipp Nagler - , Universität Regensburg (Autor:in)
  • Ashish Arora - , Westfälische Wilhelms-Universität Münster (Autor:in)
  • Robert Schmidt - , Westfälische Wilhelms-Universität Münster (Autor:in)
  • Alexey Chernikov - , Universität Regensburg (Autor:in)
  • John Lupton - , Universität Regensburg (Autor:in)
  • Rudolf Bratschitsch - , Westfälische Wilhelms-Universität Münster (Autor:in)
  • Christian Schüller - , Universität Regensburg (Autor:in)
  • Tobias Korn - , Universität Regensburg (Autor:in)

Abstract

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these semiconducting materials, optically excited electron–hole pairs form tightly Coulomb-bound excitons with large binding energies. The selection rules for excitonic transitions allow for direct optical generation of a valley-polarized exciton population using resonant excitation. Here, we investigate the exciton valley dynamics in monolayers of three different TMDCs by means of time-resolved Kerr rotation at low temperatures. We observe pronounced differences in the valley dynamics of tungsten- and molybdenum-based TMDCs, which are directly related to the opposite order of the conduction-band spin splitting in these materials.

Details

OriginalspracheEnglisch
Aufsatznummer1700131
FachzeitschriftPhysica Status Solidi - Rapid Research Letters
Jahrgang11
Ausgabenummer7
PublikationsstatusVeröffentlicht - Juli 2017
Peer-Review-StatusJa
Extern publiziertJa

Schlagworte

Schlagwörter

  • excitons, transition metal dichalcogenides, two-dimensional materials, valley dynamics, valleytronics