Valley dynamics of excitons in monolayer dichalcogenides
Publikation: Beitrag in Fachzeitschrift › Forschungsartikel › Beigetragen › Begutachtung
Beitragende
Abstract
Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these semiconducting materials, optically excited electron–hole pairs form tightly Coulomb-bound excitons with large binding energies. The selection rules for excitonic transitions allow for direct optical generation of a valley-polarized exciton population using resonant excitation. Here, we investigate the exciton valley dynamics in monolayers of three different TMDCs by means of time-resolved Kerr rotation at low temperatures. We observe pronounced differences in the valley dynamics of tungsten- and molybdenum-based TMDCs, which are directly related to the opposite order of the conduction-band spin splitting in these materials.
Details
Originalsprache | Englisch |
---|---|
Aufsatznummer | 1700131 |
Fachzeitschrift | Physica Status Solidi - Rapid Research Letters |
Jahrgang | 11 |
Ausgabenummer | 7 |
Publikationsstatus | Veröffentlicht - Juli 2017 |
Peer-Review-Status | Ja |
Extern publiziert | Ja |
Schlagworte
ASJC Scopus Sachgebiete
Schlagwörter
- excitons, transition metal dichalcogenides, two-dimensional materials, valley dynamics, valleytronics