Unraveling exciton dynamics in an atomically thin van der Waals magnet

Research output: Contribution to book/Conference proceedings/Anthology/ReportConference contributionContributedpeer-review

Contributors

Abstract

Within the realm of atomically thin semiconductors, CrSBr stands out uniquely as it harbors quasi-one-dimensional magnetic excitons in both its bulk and monolayer forms. Despite its fundamental significance, the precise exciton formation, relaxation and decay dynamics remained elusive. While terahertz polarization probing offers a direct avenue for tracking excitons, the resulting far-field signal can be affected by signals originating beyond the lateral dimensions of the sample. Here, we combine terahertz polarization spectroscopy with near-field microscopy to unveil the sub-picosecond decay dynamics of paramagnetic excitons in a CrSBr monolayer, which is faster by a factor of 30 than its bulk counterpart. Our analysis also unravels low-energy fingerprints of bound and unbound electron-hole pairs in bulk and gives access to the non-equilibrium dielectric function of the monolayer. These findings provide direct insight into the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, with potential applications in quantum devices leveraging ultrathin van der Waals magnets.

Details

Original languageEnglish
Title of host publication2024 49th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2024
PublisherInstitute of Electrical and Electronics Engineers (IEEE)
Number of pages2
ISBN (electronic)979-8-3503-7032-4
ISBN (print)979-8-3503-7033-1
Publication statusPublished - 7 Oct 2024
Peer-reviewedYes

Publication series

SeriesInternational Conference on Infrared and Millimeter Waves
ISSN2162-2027

Conference

Title49th International Conference on Infrared, Millimeter, and Terahertz Waves 2024
Abbreviated titleIRMMW-THz 2024
Conference number49
Duration1 - 6 September 2024
Website
LocationUniversity Club of Western Australia
CityPerth
CountryAustralia

External IDs

ORCID /0000-0002-9213-2777/work/196666294

Keywords

Keywords

  • Atomically thin solids, femtosecond near-field microscopy, ultrafast dynamics, van der Waals magnets