Unraveling exciton dynamics in an atomically thin van der Waals magnet
Research output: Contribution to book/Conference proceedings/Anthology/Report › Conference contribution › Contributed › peer-review
Contributors
Abstract
Within the realm of atomically thin semiconductors, CrSBr stands out uniquely as it harbors quasi-one-dimensional magnetic excitons in both its bulk and monolayer forms. Despite its fundamental significance, the precise exciton formation, relaxation and decay dynamics remained elusive. While terahertz polarization probing offers a direct avenue for tracking excitons, the resulting far-field signal can be affected by signals originating beyond the lateral dimensions of the sample. Here, we combine terahertz polarization spectroscopy with near-field microscopy to unveil the sub-picosecond decay dynamics of paramagnetic excitons in a CrSBr monolayer, which is faster by a factor of 30 than its bulk counterpart. Our analysis also unravels low-energy fingerprints of bound and unbound electron-hole pairs in bulk and gives access to the non-equilibrium dielectric function of the monolayer. These findings provide direct insight into the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, with potential applications in quantum devices leveraging ultrathin van der Waals magnets.
Details
| Original language | English |
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| Title of host publication | 2024 49th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2024 |
| Publisher | Institute of Electrical and Electronics Engineers (IEEE) |
| Number of pages | 2 |
| ISBN (electronic) | 979-8-3503-7032-4 |
| ISBN (print) | 979-8-3503-7033-1 |
| Publication status | Published - 7 Oct 2024 |
| Peer-reviewed | Yes |
Publication series
| Series | International Conference on Infrared and Millimeter Waves |
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| ISSN | 2162-2027 |
Conference
| Title | 49th International Conference on Infrared, Millimeter, and Terahertz Waves 2024 |
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| Abbreviated title | IRMMW-THz 2024 |
| Conference number | 49 |
| Duration | 1 - 6 September 2024 |
| Website | |
| Location | University Club of Western Australia |
| City | Perth |
| Country | Australia |
External IDs
| ORCID | /0000-0002-9213-2777/work/196666294 |
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Keywords
ASJC Scopus subject areas
Keywords
- Atomically thin solids, femtosecond near-field microscopy, ultrafast dynamics, van der Waals magnets