Unraveling exciton dynamics in an atomically thin van der Waals magnet

Publikation: Beitrag in Buch/Konferenzbericht/Sammelband/GutachtenBeitrag in KonferenzbandBeigetragenBegutachtung

Beitragende

Abstract

Within the realm of atomically thin semiconductors, CrSBr stands out uniquely as it harbors quasi-one-dimensional magnetic excitons in both its bulk and monolayer forms. Despite its fundamental significance, the precise exciton formation, relaxation and decay dynamics remained elusive. While terahertz polarization probing offers a direct avenue for tracking excitons, the resulting far-field signal can be affected by signals originating beyond the lateral dimensions of the sample. Here, we combine terahertz polarization spectroscopy with near-field microscopy to unveil the sub-picosecond decay dynamics of paramagnetic excitons in a CrSBr monolayer, which is faster by a factor of 30 than its bulk counterpart. Our analysis also unravels low-energy fingerprints of bound and unbound electron-hole pairs in bulk and gives access to the non-equilibrium dielectric function of the monolayer. These findings provide direct insight into the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, with potential applications in quantum devices leveraging ultrathin van der Waals magnets.

Details

OriginalspracheEnglisch
Titel2024 49th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2024
Herausgeber (Verlag)Institute of Electrical and Electronics Engineers (IEEE)
Seitenumfang2
ISBN (elektronisch)979-8-3503-7032-4
ISBN (Print)979-8-3503-7033-1
PublikationsstatusVeröffentlicht - 7 Okt. 2024
Peer-Review-StatusJa

Publikationsreihe

ReiheInternational Conference on Infrared and Millimeter Waves
ISSN2162-2027

Konferenz

Titel49th International Conference on Infrared, Millimeter, and Terahertz Waves 2024
KurztitelIRMMW-THz 2024
Veranstaltungsnummer49
Dauer1 - 6 September 2024
Webseite
OrtUniversity Club of Western Australia
StadtPerth
LandAustralien

Externe IDs

ORCID /0000-0002-9213-2777/work/196666294

Schlagworte

Schlagwörter

  • Atomically thin solids, femtosecond near-field microscopy, ultrafast dynamics, van der Waals magnets