Unraveling exciton dynamics in an atomically thin van der Waals magnet
Publikation: Beitrag in Buch/Konferenzbericht/Sammelband/Gutachten › Beitrag in Konferenzband › Beigetragen › Begutachtung
Beitragende
Abstract
Within the realm of atomically thin semiconductors, CrSBr stands out uniquely as it harbors quasi-one-dimensional magnetic excitons in both its bulk and monolayer forms. Despite its fundamental significance, the precise exciton formation, relaxation and decay dynamics remained elusive. While terahertz polarization probing offers a direct avenue for tracking excitons, the resulting far-field signal can be affected by signals originating beyond the lateral dimensions of the sample. Here, we combine terahertz polarization spectroscopy with near-field microscopy to unveil the sub-picosecond decay dynamics of paramagnetic excitons in a CrSBr monolayer, which is faster by a factor of 30 than its bulk counterpart. Our analysis also unravels low-energy fingerprints of bound and unbound electron-hole pairs in bulk and gives access to the non-equilibrium dielectric function of the monolayer. These findings provide direct insight into the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, with potential applications in quantum devices leveraging ultrathin van der Waals magnets.
Details
| Originalsprache | Englisch |
|---|---|
| Titel | 2024 49th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2024 |
| Herausgeber (Verlag) | Institute of Electrical and Electronics Engineers (IEEE) |
| Seitenumfang | 2 |
| ISBN (elektronisch) | 979-8-3503-7032-4 |
| ISBN (Print) | 979-8-3503-7033-1 |
| Publikationsstatus | Veröffentlicht - 7 Okt. 2024 |
| Peer-Review-Status | Ja |
Publikationsreihe
| Reihe | International Conference on Infrared and Millimeter Waves |
|---|---|
| ISSN | 2162-2027 |
Konferenz
| Titel | 49th International Conference on Infrared, Millimeter, and Terahertz Waves 2024 |
|---|---|
| Kurztitel | IRMMW-THz 2024 |
| Veranstaltungsnummer | 49 |
| Dauer | 1 - 6 September 2024 |
| Webseite | |
| Ort | University Club of Western Australia |
| Stadt | Perth |
| Land | Australien |
Externe IDs
| ORCID | /0000-0002-9213-2777/work/196666294 |
|---|
Schlagworte
ASJC Scopus Sachgebiete
Schlagwörter
- Atomically thin solids, femtosecond near-field microscopy, ultrafast dynamics, van der Waals magnets