Unconventional spin dynamics in the honeycomb-lattice material α-RuCl3: High-field electron spin resonance studies
Research output: Contribution to journal › Research article › Contributed › peer-review
Contributors
Abstract
We present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material α-RuCl3, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered phase, with magnetic field applied in the ab plane. A very rich excitation spectrum was observed in the field-induced quantum paramagnetic phase. The obtained data are compared with the results of recent numerical calculations, strongly suggesting a very unconventional multiparticle character of the spin dynamics in α-RuCl3. The frequency-field diagram of the lowest-energy ESR mode is found consistent with the behavior of the field-induced energy gap, revealed by thermodynamic measurements.
Details
Original language | English |
---|---|
Article number | 241107 |
Journal | Physical Review B |
Volume | 96 |
Issue number | 24 |
Publication status | Published - 19 Dec 2017 |
Peer-reviewed | Yes |