Unconventional spin dynamics in the honeycomb-lattice material α-RuCl3: High-field electron spin resonance studies

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • A. N. Ponomaryov - , Helmholtz-Zentrum Dresden-Rossendorf (Autor:in)
  • E. Schulze - , Professur für Physik in hohen Magnetfeldern (gB/HZDR), Helmholtz-Zentrum Dresden-Rossendorf (Autor:in)
  • J. Wosnitza - , Professur für Physik in hohen Magnetfeldern (gB/HZDR), Helmholtz-Zentrum Dresden-Rossendorf (Autor:in)
  • P. Lampen-Kelley - , Oak Ridge National Laboratory, University of Tennessee, Knoxville (Autor:in)
  • A. Banerjee - , Oak Ridge National Laboratory (Autor:in)
  • J. Q. Yan - , Oak Ridge National Laboratory (Autor:in)
  • C. A. Bridges - , Oak Ridge National Laboratory (Autor:in)
  • D. G. Mandrus - , Oak Ridge National Laboratory (Autor:in)
  • S. E. Nagler - , Oak Ridge National Laboratory (Autor:in)
  • A. K. Kolezhuk - , Kyiv National Taras Shevchenko University, NASU - Institute of Magnetism of NAS and MES of Ukraine (Autor:in)
  • S. A. Zvyagin - , Helmholtz-Zentrum Dresden-Rossendorf (Autor:in)

Abstract

We present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material α-RuCl3, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered phase, with magnetic field applied in the ab plane. A very rich excitation spectrum was observed in the field-induced quantum paramagnetic phase. The obtained data are compared with the results of recent numerical calculations, strongly suggesting a very unconventional multiparticle character of the spin dynamics in α-RuCl3. The frequency-field diagram of the lowest-energy ESR mode is found consistent with the behavior of the field-induced energy gap, revealed by thermodynamic measurements.

Details

OriginalspracheEnglisch
Aufsatznummer241107
FachzeitschriftPhysical Review B
Jahrgang96
Ausgabenummer24
PublikationsstatusVeröffentlicht - 19 Dez. 2017
Peer-Review-StatusJa