Ultraconfined terahertz phonon polaritons in hafnium dichalcogenides

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

Abstract

The confinement of electromagnetic radiation to subwavelength scales relies on strong light–matter interactions. In the infrared and terahertz spectral ranges, phonon polaritons are commonly employed to achieve deeply subdiffractional light confinement, with such optical modes offering much lower losses in comparison to plasmon polaritons. Among these, hyperbolic phonon polaritons in anisotropic materials offer a promising platform for light confinement. Here we report on ultraconfined phonon polaritons in hafnium-based dichalcogenides with confinement factors exceeding λ0/250 in the terahertz spectral range. This extreme light compression within deeply subwavelength thin films is enabled by the large magnitude of the light–matter coupling strength in these compounds and the natural hyperbolicity of HfSe2. Our findings emphasize the role of light–matter coupling for polariton confinement, which for phonon polaritons in polar dielectrics is dictated by the transverse–longitudinal optical phonon energy splitting. Our results demonstrate transition-metal dichalcogenides as an enabling platform for terahertz nanophotonic applications.

Details

Original languageEnglish
Pages (from-to)1735-1741
Number of pages7
JournalNature materials
Volume24
Issue number11
Early online date15 Sept 2025
Publication statusPublished - Nov 2025
Peer-reviewedYes

External IDs

ORCID /0000-0002-2484-4158/work/193175525
PubMed 40954206