Terahertz signatures of ultrafast Dirac fermion relaxation at the surface of topological insulators

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • S. Kovalev - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • K. J. Tielrooij - , Catalan Institute of Nanoscience and Nanotechnology (Author)
  • J. C. Deinert - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • I. Ilyakov - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • N. Awari - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • M. Chen - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • A. Ponomaryov - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • M. Bawatna - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • T. V.A.G. de Oliveira - , TUD Dresden University of Technology, Würzburg-Dresden Cluster of Excellence ct.qmat (Author)
  • L. M. Eng - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Experimental Physics / Photophysics, TUD Dresden University of Technology (Author)
  • K. A. Kuznetsov - , Lomonosov Moscow State University (Author)
  • D. A. Safronenkov - , Lomonosov Moscow State University (Author)
  • G. Kh Kitaeva - , Lomonosov Moscow State University (Author)
  • P. I. Kuznetsov - , National Research University of Electronic Technology (Author)
  • H. A. Hafez - , Bielefeld University (Author)
  • D. Turchinovich - , Bielefeld University (Author)
  • M. Gensch - , German Aerospace Center (DLR), Technical University of Berlin (Author)

Abstract

Topologically protected surface states present rich physics and promising spintronic, optoelectronic, and photonic applications that require a proper understanding of their ultrafast carrier dynamics. Here, we investigate these dynamics in topological insulators (TIs) of the bismuth and antimony chalcogenide family, where we isolate the response of Dirac fermions at the surface from the response of bulk carriers by combining photoexcitation with below-bandgap terahertz (THz) photons and TI samples with varying Fermi level, including one sample with the Fermi level located within the bandgap. We identify distinctly faster relaxation of charge carriers in the topologically protected Dirac surface states (few hundred femtoseconds), compared to bulk carriers (few picoseconds). In agreement with such fast cooling dynamics, we observe THz harmonic generation without any saturation effects for increasing incident fields, unlike graphene which exhibits strong saturation. This opens up promising avenues for increased THz nonlinear conversion efficiencies, and high-bandwidth optoelectronic and spintronic information and communication applications.

Details

Original languageEnglish
Article number84
Journalnpj quantum materials
Volume6
Issue number1
Publication statusPublished - Dec 2021
Peer-reviewedYes

External IDs

ORCID /0000-0002-2484-4158/work/142257566