Process intensification of gas–liquid downflow and upflow packed beds by a new low-shear rotating reactor concept

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Amir Motamed Dashliborun - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Université Laval (Author)
  • Hans Ulrich Härting - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Markus Schubert - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Faïçal Larachi - , Université Laval (Author)

Abstract

In the present work, a new low-shear rotating reactor concept was introduced for process intensification of heterogeneous catalytic reactions in cocurrent gas–liquid downflow and upflow packed-bed reactors. To properly assess potential advantages of this new reactor concept, exhaustive hydrodynamic experiments were carried out using embedded low-intrusive wire mesh sensors. The effect of the rotational velocity on liquid flow patterns in the bed cross-section, liquid saturation, pressure drop, and regime transition was investigated. Furthermore, liquid residence time and Péclet number estimated by a stimulus-response technique and a macro-mixing model were presented and discussed with respect to the prevailing flow patterns. The results revealed that the column rotation induces different flow patterns in the cross-section of the packed bed operating in a concurrent downflow or upflow mode. Moreover, the new reactor concept exhibits a more flexible adjustment of pressure drop, liquid saturation, liquid residence time, and back-mixing at constant flow rates.

Details

Original languageEnglish
Pages (from-to)283-294
Number of pages12
JournalAIChE Journal
Volume63
Issue number1
Publication statusPublished - 1 Jan 2017
Peer-reviewedYes
Externally publishedYes

Keywords

Keywords

  • downflow and upflow, flow pattern, hydrodynamics, low-shear rotating fixed bed, process intensification