Process intensification of gas–liquid downflow and upflow packed beds by a new low-shear rotating reactor concept

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Amir Motamed Dashliborun - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Université Laval (Autor:in)
  • Hans Ulrich Härting - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Markus Schubert - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Faïçal Larachi - , Université Laval (Autor:in)

Abstract

In the present work, a new low-shear rotating reactor concept was introduced for process intensification of heterogeneous catalytic reactions in cocurrent gas–liquid downflow and upflow packed-bed reactors. To properly assess potential advantages of this new reactor concept, exhaustive hydrodynamic experiments were carried out using embedded low-intrusive wire mesh sensors. The effect of the rotational velocity on liquid flow patterns in the bed cross-section, liquid saturation, pressure drop, and regime transition was investigated. Furthermore, liquid residence time and Péclet number estimated by a stimulus-response technique and a macro-mixing model were presented and discussed with respect to the prevailing flow patterns. The results revealed that the column rotation induces different flow patterns in the cross-section of the packed bed operating in a concurrent downflow or upflow mode. Moreover, the new reactor concept exhibits a more flexible adjustment of pressure drop, liquid saturation, liquid residence time, and back-mixing at constant flow rates.

Details

OriginalspracheEnglisch
Seiten (von - bis)283-294
Seitenumfang12
FachzeitschriftAIChE Journal
Jahrgang63
Ausgabenummer1
PublikationsstatusVeröffentlicht - 1 Jan. 2017
Peer-Review-StatusJa
Extern publiziertJa

Schlagworte

Schlagwörter

  • downflow and upflow, flow pattern, hydrodynamics, low-shear rotating fixed bed, process intensification