Polaronic conductivity in the photoinduced phase of 1T-TaS2

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • N. Dean - , University of Oxford (Author)
  • J. C. Petersen - , University of Oxford, University of Hamburg (Author)
  • D. Fausti - , University of Oxford, University of Hamburg (Author)
  • R. I. Tobey - , University of Oxford, Brookhaven National Laboratory (Author)
  • S. Kaiser - , Max Planck Institute for the Structure and Dynamics of Matter, University of Hamburg (Author)
  • L. V. Gasparov - , University of North Florida (Author)
  • H. Berger - , Swiss Federal Institute of Technology Lausanne (EPFL) (Author)
  • A. Cavalleri - , University of Oxford, University of Hamburg (Author)

Abstract

The transient optical conductivity of photoexcited 1T-TaS2 is determined over a three-order-of-magnitude frequency range. Prompt collapse and recovery of the Mott gap is observed. However, we find important differences between this transient metallic state and that seen across the thermally driven insulator-metal transition. Suppressed low-frequency conductivity, Fano phonon line shapes, and a midinfrared absorption band point to polaronic transport. This is explained by noting that the photoinduced metallic state of 1T-TaS 2 is one in which the Mott gap is melted but the lattice retains its low-temperature symmetry, a regime only accessible by photodoping.

Details

Original languageEnglish
Article number016401
JournalPhysical review letters
Volume106
Issue number1
Publication statusPublished - 4 Jan 2011
Peer-reviewedYes
Externally publishedYes

External IDs

ORCID /0000-0001-9862-2788/work/142255391

Keywords

ASJC Scopus subject areas