Polaronic conductivity in the photoinduced phase of 1T-TaS2

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • N. Dean - , University of Oxford (Autor:in)
  • J. C. Petersen - , University of Oxford, Universität Hamburg (Autor:in)
  • D. Fausti - , University of Oxford, Universität Hamburg (Autor:in)
  • R. I. Tobey - , University of Oxford, Brookhaven National Laboratory (Autor:in)
  • S. Kaiser - , Max Planck Institute for the Structure and Dynamics of Matter, Universität Hamburg (Autor:in)
  • L. V. Gasparov - , University of North Florida (Autor:in)
  • H. Berger - , École Polytechnique Fédérale de Lausanne (Autor:in)
  • A. Cavalleri - , University of Oxford, Universität Hamburg (Autor:in)

Abstract

The transient optical conductivity of photoexcited 1T-TaS2 is determined over a three-order-of-magnitude frequency range. Prompt collapse and recovery of the Mott gap is observed. However, we find important differences between this transient metallic state and that seen across the thermally driven insulator-metal transition. Suppressed low-frequency conductivity, Fano phonon line shapes, and a midinfrared absorption band point to polaronic transport. This is explained by noting that the photoinduced metallic state of 1T-TaS 2 is one in which the Mott gap is melted but the lattice retains its low-temperature symmetry, a regime only accessible by photodoping.

Details

OriginalspracheEnglisch
Aufsatznummer016401
FachzeitschriftPhysical review letters
Jahrgang106
Ausgabenummer1
PublikationsstatusVeröffentlicht - 4 Jan. 2011
Peer-Review-StatusJa
Extern publiziertJa

Externe IDs

ORCID /0000-0001-9862-2788/work/142255391

Schlagworte

ASJC Scopus Sachgebiete