Paratellurite Nanowires as a Versatile Material for THz Phonon Polaritons

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

Abstract

Polaritons, i.e., hybrid quasi-particles of light and matter resonances, have been extensively investigated due to their potential to enhance light-matter interactions. Although polaritonic applications thrive in the mid-infrared range, their extension to the terahertz (THz) range remains limited. Here, we present paratellurite (α-TeO2) nanowires, a versatile material acting as a platform for different types of phonon polaritons. Utilizing synchrotron infrared nanospectroscopy from 10 to 24 THz, we uncover the polaritonic properties of α-TeO2 nanowires, showcasing their dual functionality as both a Fabry-Pérot cavity and a waveguide for surface phonon polaritons. Furthermore, near-field measurements with a free-electron laser as a THz source reveal a localized optical contrast down to 5.5 THz, an indication of hyperbolic bands. Our findings complement the repertoire of polaritonic materials, with significant implications for advancing THz technologies.

Details

Original languageEnglish
Pages (from-to)4323-4333
Number of pages11
JournalACS Photonics
Volume11
Issue number10
Publication statusPublished - 20 Sept 2024
Peer-reviewedYes

External IDs

ORCID /0000-0002-2484-4158/work/168205142

Keywords