Orbital order induced ferromagnetic insulating properties

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • J. Geck - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • P. Wochner - , Max Planck Institute for Intelligent Systems (Author)
  • S. Kiele - , Leibniz Institute for Solid State and Materials Research Dresden, German Electron Synchrotron (DESY) (Author)
  • R. Klingeler - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • A. Revcolevschi - , French National Centre for Scientific Research (CNRS) (Author)
  • M. V. Zimmermann - , German Electron Synchrotron (DESY) (Author)
  • B. Büchner - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • P. Reutler - , French National Centre for Scientific Research (CNRS) (Author)

Abstract

At temperatures below the metal-insulator transition of La 1-xSrxMnO3 with 0.1 < x < 0.15, a peculiar ferromagnetic and insulating phase is observed which has been intensively discussed over the last few years. We present a detailed investigation of this phase by means of resonant and high energy x-ray scattering along with measurements of the electrical resistivity, thermal expansion, magnetization, and specific heat. Interestingly, the data show that the metal-insulator transition of lightly doped manganites is accompanied by an orbital rearrangement. The microscopic information provided by the x-ray scattering studies together with the analysis of the macroscopic properties implies that the orbital reordering maximizes the gain of double exchange energy and, at the same time, induces an insulating behaviour. The relevance of the double-exchange mechanism for the stabilization of the ferromagnetic insulating phase is further substantiated by studies of (La1-yPr y)7/8Sr1/8MnO3: with increasing praseodymium content, the metal-insulator transition is dramatically suppressed which can naturally be explained by a reduction of the band width upon praseodymium doping.

Details

Original languageEnglish
Pages (from-to)1-27
Number of pages27
JournalNew journal of physics
Volume6
Publication statusPublished - 5 Nov 2004
Peer-reviewedYes

External IDs

ORCID /0000-0002-2438-0672/work/158767797

Keywords

ASJC Scopus subject areas