Orbital order induced ferromagnetic insulating properties

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • J. Geck - , Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • P. Wochner - , Max-Planck-Institut für Intelligente Systeme (Autor:in)
  • S. Kiele - , Leibniz Institute for Solid State and Materials Research Dresden, Deutsches Elektronen-Synchrotron (DESY) (Autor:in)
  • R. Klingeler - , Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • A. Revcolevschi - , Centre national de la recherche scientifique (CNRS) (Autor:in)
  • M. V. Zimmermann - , Deutsches Elektronen-Synchrotron (DESY) (Autor:in)
  • B. Büchner - , Professur für Experimentelle Festkörperphysik (gB/IFW), Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • P. Reutler - , Centre national de la recherche scientifique (CNRS) (Autor:in)

Abstract

At temperatures below the metal-insulator transition of La 1-xSrxMnO3 with 0.1 < x < 0.15, a peculiar ferromagnetic and insulating phase is observed which has been intensively discussed over the last few years. We present a detailed investigation of this phase by means of resonant and high energy x-ray scattering along with measurements of the electrical resistivity, thermal expansion, magnetization, and specific heat. Interestingly, the data show that the metal-insulator transition of lightly doped manganites is accompanied by an orbital rearrangement. The microscopic information provided by the x-ray scattering studies together with the analysis of the macroscopic properties implies that the orbital reordering maximizes the gain of double exchange energy and, at the same time, induces an insulating behaviour. The relevance of the double-exchange mechanism for the stabilization of the ferromagnetic insulating phase is further substantiated by studies of (La1-yPr y)7/8Sr1/8MnO3: with increasing praseodymium content, the metal-insulator transition is dramatically suppressed which can naturally be explained by a reduction of the band width upon praseodymium doping.

Details

OriginalspracheEnglisch
Seiten (von - bis)1-27
Seitenumfang27
FachzeitschriftNew journal of physics
Jahrgang6
PublikationsstatusVeröffentlicht - 5 Nov. 2004
Peer-Review-StatusJa

Externe IDs

ORCID /0000-0002-2438-0672/work/158767797

Schlagworte

ASJC Scopus Sachgebiete