Nonlinear plasmonic response of doped nanowires observed by infrared nanospectroscopy
Research output: Contribution to journal › Research article › Contributed › peer-review
Contributors
Abstract
We report a strong shift of the plasma resonance in highly-doped GaAs/InGaAs core/shell nanowires (NWs) for intense infrared excitation observed by scattering-type scanning near-field infrared microscopy. The studied NWs show a sharp plasma resonance at a photon energy of about 125 meV in the case of continuous wave excitation by a CO 2 laser. Probing the same NWs with the pulsed free-electron laser with peak electric field strengths up to several 10 kV cm -1 reveals a power-dependent redshift to about 95 meV and broadening of the plasmonic resonance. We assign this effect to a substantial heating of the electrons in the conduction band and subsequent increase of the effective mass in the nonparabolic Γ-valley.
Details
Original language | English |
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Article number | 084003 |
Journal | Nanotechnology |
Volume | 30 |
Issue number | 8 |
Publication status | Published - 22 Feb 2019 |
Peer-reviewed | Yes |
External IDs
PubMed | 30523880 |
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ORCID | /0000-0002-2484-4158/work/158768080 |
Keywords
ASJC Scopus subject areas
Keywords
- free-electron laser, infrared nanospectroscopy, nanowires, nonlinear plasmonics, InGaAs, s-SNIM