Intermixing-Driven Surface and Bulk Ferromagnetism in the Quantum Anomalous Hall Candidate MnBi6Te10

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Abdul Vakhab Tcakaev - , University of Würzburg, Würzburg-Dresden Cluster of Excellence ct.qmat (Author)
  • Bastian Rubrecht - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Jorge I. Facio - , Leibniz Institute for Solid State and Materials Research Dresden, Comisión Nacional de Energía Atómica (Author)
  • Volodymyr B. Zabolotnyy - , University of Würzburg, Würzburg-Dresden Cluster of Excellence ct.qmat (Author)
  • Laura T. Corredor - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Laura C. Folkers - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Junior Professorship in Synthesis and Crystal Growth of Quantum Materials (Author)
  • Ekaterina Kochetkova - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Thiago R.F. Peixoto - , Würzburg-Dresden Cluster of Excellence ct.qmat, University of Würzburg (Author)
  • Philipp Kagerer - , Würzburg-Dresden Cluster of Excellence ct.qmat, University of Würzburg (Author)
  • Simon Heinze - , Heidelberg University  (Author)
  • Hendrik Bentmann - , Würzburg-Dresden Cluster of Excellence ct.qmat, University of Würzburg (Author)
  • Robert J. Green - , University of British Columbia, University of Saskatchewan (Author)
  • Pierluigi Gargiani - , Autonomous University of Barcelona (Author)
  • Manuel Valvidares - , Autonomous University of Barcelona (Author)
  • Eugen Weschke - , Helmholtz Centre Berlin for Materials and Energy (Author)
  • Maurits W. Haverkort - , Heidelberg University  (Author)
  • Friedrich Reinert - , Würzburg-Dresden Cluster of Excellence ct.qmat, University of Würzburg (Author)
  • Jeroen van den Brink - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Solid State Theory, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Bernd Büchner - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Anja U.B. Wolter - , Würzburg-Dresden Cluster of Excellence ct.qmat, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Anna Isaeva - , Leibniz Institute for Solid State and Materials Research Dresden, University of Amsterdam (Author)
  • Vladimir Hinkov - , University of Würzburg, Würzburg-Dresden Cluster of Excellence ct.qmat (Author)

Abstract

The recent realizations of the quantum anomalous Hall effect (QAHE) in MnBi2Te4 and MnBi4Te7 benchmark the (MnBi2Te4)(Bi2Te3)n family as a promising hotbed for further QAHE improvements. The family owes its potential to its ferromagnetically (FM) ordered MnBi2Te4 septuple layers (SLs). However, the QAHE realization is complicated in MnBi2Te4 and MnBi4Te7 due to the substantial antiferromagnetic (AFM) coupling between the SLs. An FM state, advantageous for the QAHE, can be stabilized by interlacing the SLs with an increasing number n of Bi2Te3 quintuple layers (QLs). However, the mechanisms driving the FM state and the number of necessary QLs are not understood, and the surface magnetism remains obscure. Here, robust FM properties in MnBi6Te10 (n = 2) with Tc ≈ 12 K are demonstrated and their origin is established in the Mn/Bi intermixing phenomenon by a combined experimental and theoretical study. The measurements reveal a magnetically intact surface with a large magnetic moment, and with FM properties similar to the bulk. This investigation thus consolidates the MnBi6Te10 system as perspective for the QAHE at elevated temperatures.

Details

Original languageEnglish
Article number2203239
JournalAdvanced science
Volume10
Issue number10
Publication statusPublished - 5 Apr 2023
Peer-reviewedYes

Keywords

Keywords

  • intrinsic magnetic topological insulator, magnetic topological insulator, magnetism, superconducting quantum interference device (SQUID), topological insulator, X-ray absorption spectroscopy (XAS), X-ray magnetic circular dichroism (XMCD)