Intermixing-Driven Surface and Bulk Ferromagnetism in the Quantum Anomalous Hall Candidate MnBi6Te10

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Abdul Vakhab Tcakaev - , Julius-Maximilians-Universität Würzburg, Würzburg-Dresden Cluster of Excellence ct.qmat (Autor:in)
  • Bastian Rubrecht - , Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • Jorge I. Facio - , Leibniz Institute for Solid State and Materials Research Dresden, Comisión Nacional de Energía Atómica (Autor:in)
  • Volodymyr B. Zabolotnyy - , Julius-Maximilians-Universität Würzburg, Würzburg-Dresden Cluster of Excellence ct.qmat (Autor:in)
  • Laura T. Corredor - , Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • Laura C. Folkers - , Exzellenzcluster ct.qmat: Komplexität und Topologie in Quantenmaterialien, Juniorprofessur Synthese und Kristallzüchtung von Quantenmaterialien (Autor:in)
  • Ekaterina Kochetkova - , Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • Thiago R.F. Peixoto - , Würzburg-Dresden Cluster of Excellence ct.qmat, Julius-Maximilians-Universität Würzburg (Autor:in)
  • Philipp Kagerer - , Würzburg-Dresden Cluster of Excellence ct.qmat, Julius-Maximilians-Universität Würzburg (Autor:in)
  • Simon Heinze - , Universität Heidelberg (Autor:in)
  • Hendrik Bentmann - , Würzburg-Dresden Cluster of Excellence ct.qmat, Julius-Maximilians-Universität Würzburg (Autor:in)
  • Robert J. Green - , University of British Columbia, University of Saskatchewan (Autor:in)
  • Pierluigi Gargiani - , Autonomous University of Barcelona (Autor:in)
  • Manuel Valvidares - , Autonomous University of Barcelona (Autor:in)
  • Eugen Weschke - , Helmholtz-Zentrum Berlin für Materialien und Energie (HZB) (Autor:in)
  • Maurits W. Haverkort - , Universität Heidelberg (Autor:in)
  • Friedrich Reinert - , Würzburg-Dresden Cluster of Excellence ct.qmat, Julius-Maximilians-Universität Würzburg (Autor:in)
  • Jeroen van den Brink - , Exzellenzcluster ct.qmat: Komplexität und Topologie in Quantenmaterialien, Professur für Festkörpertheorie (gB/IFW), Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • Bernd Büchner - , Exzellenzcluster ct.qmat: Komplexität und Topologie in Quantenmaterialien, Professur für Experimentelle Festkörperphysik (gB/IFW), Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • Anja U.B. Wolter - , Würzburg-Dresden Cluster of Excellence ct.qmat, Leibniz Institute for Solid State and Materials Research Dresden (Autor:in)
  • Anna Isaeva - , Leibniz Institute for Solid State and Materials Research Dresden, University of Amsterdam (Autor:in)
  • Vladimir Hinkov - , Julius-Maximilians-Universität Würzburg, Würzburg-Dresden Cluster of Excellence ct.qmat (Autor:in)

Abstract

The recent realizations of the quantum anomalous Hall effect (QAHE) in MnBi2Te4 and MnBi4Te7 benchmark the (MnBi2Te4)(Bi2Te3)n family as a promising hotbed for further QAHE improvements. The family owes its potential to its ferromagnetically (FM) ordered MnBi2Te4 septuple layers (SLs). However, the QAHE realization is complicated in MnBi2Te4 and MnBi4Te7 due to the substantial antiferromagnetic (AFM) coupling between the SLs. An FM state, advantageous for the QAHE, can be stabilized by interlacing the SLs with an increasing number n of Bi2Te3 quintuple layers (QLs). However, the mechanisms driving the FM state and the number of necessary QLs are not understood, and the surface magnetism remains obscure. Here, robust FM properties in MnBi6Te10 (n = 2) with Tc ≈ 12 K are demonstrated and their origin is established in the Mn/Bi intermixing phenomenon by a combined experimental and theoretical study. The measurements reveal a magnetically intact surface with a large magnetic moment, and with FM properties similar to the bulk. This investigation thus consolidates the MnBi6Te10 system as perspective for the QAHE at elevated temperatures.

Details

OriginalspracheEnglisch
Aufsatznummer2203239
FachzeitschriftAdvanced science
Jahrgang10
Ausgabenummer10
PublikationsstatusVeröffentlicht - 5 Apr. 2023
Peer-Review-StatusJa

Schlagworte

Schlagwörter

  • intrinsic magnetic topological insulator, magnetic topological insulator, magnetism, superconducting quantum interference device (SQUID), topological insulator, X-ray absorption spectroscopy (XAS), X-ray magnetic circular dichroism (XMCD)