Gold nanoparticle tips for optical field confinement in infrared scattering near-field optical microscopy

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

Abstract

We report on the implementation of metal nanoparticles as probes for scattering and apertureless near-field optical investigations in the mid-infrared (mid-IR) spectral regime. At these wavelengths, an efficient electric-field confinement is necessary and achieved here through a gold metal nanoparticle of 80 nm in diameter (Au80-MNP) acting as the optical antenna. The Au80-MNP is attached to a standard AFM cantilever used as the spatial manipulator. When approached to a sample surface while being illuminated with an infrared beam, the Au80-MNP produces a considerably improved spatial confinement of the electric field compared to an ordinary scattering AFM tip. We demonstrate here the confinement normal to the sample surface by making use of a sample-induced phonon polariton resonance in a ferroelectric lithium niobate sample. Our experimental findings are in very good agreement with the quasistatic dipole model and show improved optical resolution via well-selected antenna particles.

Details

Original languageEnglish
Pages (from-to)12302-12312
Number of pages11
JournalOptics express
Volume16
Issue number16
Publication statusPublished - 4 Aug 2008
Peer-reviewedYes

External IDs

PubMed 18679508
ORCID /0000-0002-2484-4158/work/175744074

Keywords