Doping Dependence of Collective Spin and Orbital Excitations in the Spin-1 Quantum Antiferromagnet La2-xSrxNiO4 Observed by X Rays

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • G. Fabbris - , Brookhaven National Laboratory (Author)
  • D. Meyers - , Brookhaven National Laboratory (Author)
  • L. Xu - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • V. M. Katukuri - , Leibniz Institute for Solid State and Materials Research Dresden, Swiss Federal Institute of Technology Lausanne (EPFL) (Author)
  • L. Hozoi - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • X. Liu - , CAS - Chinese Academy of Sciences (Author)
  • Z. Y. Chen - , National Synchrotron Radiation Research Center Taiwan (Author)
  • J. Okamoto - , National Synchrotron Radiation Research Center Taiwan (Author)
  • T. Schmitt - , Paul Scherrer Institute (Author)
  • A. Uldry - , Paul Scherrer Institute (Author)
  • B. Delley - , Paul Scherrer Institute (Author)
  • G. D. Gu - , Brookhaven National Laboratory (Author)
  • D. Prabhakaran - , University of Oxford (Author)
  • A. T. Boothroyd - , University of Oxford (Author)
  • J. Van Den Brink - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • D. J. Huang - , National Synchrotron Radiation Research Center Taiwan, National Tsing Hua University (Author)
  • M. P.M. Dean - , Brookhaven National Laboratory (Author)

Abstract

We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to collective magnetic excitations in S=1 systems by probing the Ni L3 edge of La2-xSrxNiO4 (x=0, 0.33, 0.45). The magnetic excitation peak is asymmetric, indicating the presence of single and multi-spin-flip excitations. As the hole doping level is increased, the zone boundary magnon energy is suppressed at a much larger rate than that in hole doped cuprates. Based on the analysis of the orbital and charge excitations observed by RIXS, we argue that this difference is related to the orbital character of the doped holes in these two families. This work establishes RIXS as a probe of fundamental magnetic interactions in nickelates opening the way towards studies of heterostructures and ultrafast pump-probe experiments.

Details

Original languageEnglish
Article number156402
JournalPhysical review letters
Volume118
Issue number15
Publication statusPublished - 12 Apr 2017
Peer-reviewedYes
Externally publishedYes

External IDs

PubMed 28452512

Keywords

ASJC Scopus subject areas