Doping Dependence of Collective Spin and Orbital Excitations in the Spin-1 Quantum Antiferromagnet La2-xSrxNiO4 Observed by X Rays

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • G. Fabbris - , Brookhaven National Laboratory (Autor:in)
  • D. Meyers - , Brookhaven National Laboratory (Autor:in)
  • L. Xu - , Leibniz-Institut für Festkörper- und Werkstoffforschung Dresden (Autor:in)
  • V. M. Katukuri - , Leibniz-Institut für Festkörper- und Werkstoffforschung Dresden, École Polytechnique Fédérale de Lausanne (Autor:in)
  • L. Hozoi - , Leibniz-Institut für Festkörper- und Werkstoffforschung Dresden (Autor:in)
  • X. Liu - , CAS - Chinese Academy of Sciences (Autor:in)
  • Z. Y. Chen - , National Synchrotron Radiation Research Center Taiwan (Autor:in)
  • J. Okamoto - , National Synchrotron Radiation Research Center Taiwan (Autor:in)
  • T. Schmitt - , Paul Scherrer Institute (Autor:in)
  • A. Uldry - , Paul Scherrer Institute (Autor:in)
  • B. Delley - , Paul Scherrer Institute (Autor:in)
  • G. D. Gu - , Brookhaven National Laboratory (Autor:in)
  • D. Prabhakaran - , University of Oxford (Autor:in)
  • A. T. Boothroyd - , University of Oxford (Autor:in)
  • J. Van Den Brink - , Leibniz-Institut für Festkörper- und Werkstoffforschung Dresden (Autor:in)
  • D. J. Huang - , National Synchrotron Radiation Research Center Taiwan, National Tsing Hua University (Autor:in)
  • M. P.M. Dean - , Brookhaven National Laboratory (Autor:in)

Abstract

We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to collective magnetic excitations in S=1 systems by probing the Ni L3 edge of La2-xSrxNiO4 (x=0, 0.33, 0.45). The magnetic excitation peak is asymmetric, indicating the presence of single and multi-spin-flip excitations. As the hole doping level is increased, the zone boundary magnon energy is suppressed at a much larger rate than that in hole doped cuprates. Based on the analysis of the orbital and charge excitations observed by RIXS, we argue that this difference is related to the orbital character of the doped holes in these two families. This work establishes RIXS as a probe of fundamental magnetic interactions in nickelates opening the way towards studies of heterostructures and ultrafast pump-probe experiments.

Details

OriginalspracheEnglisch
Aufsatznummer156402
FachzeitschriftPhysical review letters
Jahrgang118
Ausgabenummer15
PublikationsstatusVeröffentlicht - 12 Apr. 2017
Peer-Review-StatusJa
Extern publiziertJa

Externe IDs

PubMed 28452512

Schlagworte

ASJC Scopus Sachgebiete