Crossover from Collective to Incoherent Spin Excitations in Superconducting Cuprates Probed by Detuned Resonant Inelastic X-Ray Scattering
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Contributors
Abstract
Spin excitations in the overdoped high temperature superconductors Tl2Ba2CuO6+δ and (Bi,Pb)2(Sr,La)2CuO6+δ were investigated by resonant inelastic x-ray scattering (RIXS) as functions of doping and detuning of the incoming photon energy above the Cu−L₃ absorption peak. The RIXS spectra at optimal doping are dominated by a paramagnon feature with peak energy independent of photon energy, similar to prior results on underdoped cuprates. Beyond optimal doping, the RIXS data indicate a sharp crossover to a regime with a strong contribution from incoherent particle-hole excitations whose maximum shows a fluorescencelike shift upon detuning. The spectra of both compound families are closely similar, and their salient features are reproduced by exact-diagonalization calculations of the single-band Hubbard model on a finite cluster. The results are discussed in the light of recent transport experiments indicating a quantum phase transition near optimal doping.
Details
Original language | English |
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Article number | 097001 |
Journal | Physical review letters |
Volume | 119 |
Publication status | Published - 31 Aug 2017 |
Peer-reviewed | Yes |
Externally published | Yes |
External IDs
Scopus | 85029702202 |
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