Understanding unconventional magnetic order in a candidate axion insulator by resonant elastic x-ray scattering

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Jian Rui Soh - , Swiss Federal Institute of Technology Lausanne (EPFL) (Author)
  • Alessandro Bombardi - , Diamond Light Source (Author)
  • Frédéric Mila - , Swiss Federal Institute of Technology Lausanne (EPFL) (Author)
  • Marein C. Rahn - , Chair of Physics of Quantum Materials, TUD Dresden University of Technology (Author)
  • Dharmalingam Prabhakaran - , University of Oxford (Author)
  • Sonia Francoual - , German Electron Synchrotron (DESY) (Author)
  • Henrik M. Rønnow - , Swiss Federal Institute of Technology Lausanne (EPFL) (Author)
  • Andrew T. Boothroyd - , University of Oxford (Author)

Abstract

Magnetic topological insulators and semimetals are a class of crystalline solids whose properties are strongly influenced by the coupling between non-trivial electronic topology and magnetic spin configurations. Such materials can host exotic electromagnetic responses. Among these are topological insulators with certain types of antiferromagnetic order which are predicted to realize axion electrodynamics. Here we investigate the highly unusual helimagnetic phases recently reported in EuIn2As2, which has been identified as a candidate for an axion insulator. Using resonant elastic x-ray scattering we show that the two types of magnetic order observed in EuIn2As2 are spatially uniform phases with commensurate chiral magnetic structures, ruling out a possible phase-separation scenario, and we propose that entropy associated with low energy spin fluctuations plays a significant role in driving the phase transition between them. Our results establish that the magnetic order in EuIn2As2 satisfies the symmetry requirements for an axion insulator.

Details

Original languageEnglish
Article number3387
JournalNature communications
Volume14
Issue number1
Publication statusPublished - Dec 2023
Peer-reviewedYes

External IDs

PubMed 37296136