Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr
Research output: Contribution to journal › Research article › Contributed › peer-review
Contributors
Abstract
Among atomically thin semiconductors, CrSBr stands out as both its bulk and monolayer forms host tightly bound, quasi-one-dimensional excitons in a magnetic environment. Despite its pivotal importance for solid-state research, the exciton lifetime has remained unknown. While terahertz polarization probing can directly trace all excitons, independently of interband selection rules, the corresponding large far-field foci substantially exceed the lateral sample dimensions. Here, we combine terahertz polarization spectroscopy with near-field microscopy to reveal a femtosecond decay of paramagnetic excitons in a monolayer of CrSBr, which is 30 times shorter than the bulk lifetime. We unveil low-energy fingerprints of bound and unbound electron-hole pairs in bulk CrSBr and extract the nonequilibrium dielectric function of the monolayer in a model-free manner. Our results demonstrate the first direct access to the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, potentially advancing the development of quantum devices based on ultrathin van der Waals magnets.
Details
| Original language | English |
|---|---|
| Pages (from-to) | 4101-4107 |
| Number of pages | 7 |
| Journal | Nano letters |
| Volume | 24(2024) |
| Issue number | 14 |
| Publication status | Published - 10 Apr 2024 |
| Peer-reviewed | Yes |
External IDs
| PubMed | 38507732 |
|---|---|
| ORCID | /0000-0002-9213-2777/work/196666161 |
Keywords
ASJC Scopus subject areas
Keywords
- anisotropic excitons, atomically thin solids, femtosecond near-field microscopy, terahertz, ultrafast dynamics, van der Waals magnets