The vicinity of hyper-honeycomb β-Li2IrO3 to a three-dimensional Kitaev spin liquid state

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Contributors

  • Vamshi M. Katukuri - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Ravi Yadav - , Chair of Solid State Theory, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Liviu Hozoi - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Satoshi Nishimoto - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Jeroen Van Den Brink - , Chair of Solid State Theory, Leibniz Institute for Solid State and Materials Research Dresden, Harvard University (Author)

Abstract

Due to the combination of a substantial spin-orbit coupling and correlation effects, iridium oxides hold a prominent place in the search for novel quantum states of matter, including, e.g., Kitaev spin liquids and topological Weyl states. We establish the promise of the very recently synthesized hyper-honeycomb iridate β-Li2IrO3 in this regard. A detailed theoretical analysis reveals the presence of large ferromagnetic first-neighbor Kitaev interactions, while a second-neighbor antiferromagnetic Heisenberg exchange drives the ground state from ferro to zigzag order via a three-dimensional Kitaev spin liquid and an incommensurate phase. Experiment puts the system in the latter regime but the Kitaev spin liquid is very close and reachable by a slight modification of the ratio between the second- and first-neighbor couplings, for instance via strain.

Details

Original languageEnglish
Article number29585
JournalScientific reports
Volume6
Publication statusPublished - 12 Jul 2016
Peer-reviewedYes

Keywords

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