Spin-polaron ladder spectrum of the spin-orbit-induced Mott insulator Sr2IrO4 probed by scanning tunneling spectroscopy

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Jose M. Guevara - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Zhixiang Sun - , Center for Transport and Devices of Emergent Materials (CTD), Leibniz Institute for Solid State and Materials Research Dresden, Tianjin University (Author)
  • Ekaterina M. Pärschke - , Leibniz Institute for Solid State and Materials Research Dresden, University of Alabama at Birmingham (Author)
  • Steffen Sykora - , Chair of Theoretical Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Kaustuv Manna - , Leibniz Institute for Solid State and Materials Research Dresden, Max Planck Institute for Chemical Physics of Solids (Author)
  • Johannes Schoop - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Andrey Maljuk - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Sabine Wurmehl - , Leibniz Institute for Solid State and Materials Research Dresden, TUD Dresden University of Technology (Author)
  • Jeroen Van Den Brink - , Chair of Solid State Theory, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Bernd Büchner - , Center for Transport and Devices of Emergent Materials (CTD), Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden, TUD Dresden University of Technology (Author)
  • Christian Hess - , Leibniz Institute for Solid State and Materials Research Dresden, TUD Dresden University of Technology (Author)

Abstract

The motion of doped electrons or holes in an antiferromagnetic lattice with strong on-site Coulomb interactions touches one of the most fundamental open problems in contemporary condensed matter physics. The doped charge may strongly couple to elementary spin excitations, resulting in a dressed quasiparticle which is subject to confinement. This "spin polaron" possesses internal degrees of freedom with a characteristic "ladder" excitation spectrum. Despite its fundamental importance for understanding higherature superconductivity, clear experimental spectroscopic signatures of these internal degrees of freedom are scarce. Here, we present scanning tunneling spectroscopy results of the spin-orbit-induced Mott insulator Sr2IrO4. Our spectroscopy data reveal distinct shoulder-like features for occupied and unoccupied states beyond a measured Mott gap of Δ≈620 meV. Using the self-consistent Born approximation we assign the anomalies in the unoccupied states to the spin-polaron ladder spectrum with excellent quantitative agreement and estimate the Coulomb repulsion U=2.05...2.28 eV in this material. These results confirm the strongly correlated electronic structure of this compound and underpin the previously conjectured paradigm of emergent unconventional superconductivity in doped Sr2IrO4.

Details

Original languageEnglish
Article number121114
JournalPhysical Review B
Volume99
Issue number12
Publication statusPublished - 29 Mar 2019
Peer-reviewedYes