Short-Wave Infrared Optoelectronics with Colloidal CdHgSe/ZnCdS Core/Shell Nanoplatelets

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Hossein Roshan - , Italian Institute of Technology (Author)
  • Anatol Prudnikau - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Jinfei Dai - , Xi'an Jiaotong University (Author)
  • Matilde Cirignano - , Italian Institute of Technology (Author)
  • Francesco De Boni - , Italian Institute of Technology (Author)
  • Mirko Prato - , Italian Institute of Technology (Author)
  • Fabian Paulus - , Center for Advancing Electronics Dresden (cfaed), Transport in Hybrid Materials (Junior Research Group) (cfaed), Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Vladimir Lesnyak - , Chair of Physical Chemistry (Author)
  • Francesco Di Stasio - , Italian Institute of Technology (Author)

Abstract

Colloidal semiconductor nanocrystals (NCs) are an efficient and cost-effective class of nanomaterials for optoelectronic applications. Advancements in NC-based optoelectronic devices have resulted from progress in synthetic chemistry, adjustable surface properties, and optimized device architectures. Semiconductor nanoplatelets (NPLs) stand out among other NCs due to their precise growth control, yielding uniform thickness with submonolayer roughness. In this study, we demonstrate the versatility of core/shell CdxHg1-xSe/ZnyCd1-yS NPLs for optoelectronic applications in the short-wave infrared (SWIR) spectral range. We employed the very same core/shell NPLs for the fabrication of light-emitting diodes and photodetectors alike, achieving significant performance in both electroluminescence (external quantum efficiency ranging from 7.5% at 1280 nm to 3.8% at 1550 nm) and detection (responsivity of 0.24 A W-1 at 1200 nm).

Details

Original languageEnglish
Pages (from-to)40-47
Number of pages8
JournalACS photonics
Volume12
Issue number1
Publication statusPublished - 15 Jan 2025
Peer-reviewedYes

Keywords

Keywords

  • colloidal semiconductor, light-emitting diode, nanocrystals, nanoplatelets, near-infrared, photodiode, short-wave infrared