Self-Assembled Monolayers of Cyclohexyl-Terminated Phosphonic Acids as a General Dielectric Surface for High-Performance Organic Thin-Film Transistors

Research output: Contribution to journal › Research article › Contributed › peer-review

Contributors

  • Danqing Liu - , Chinese University of Hong Kong (Author)
  • Zikai He - , Chinese University of Hong Kong (Author)
  • Yaorong Su - , Chinese University of Hong Kong (Author)
  • Ying Diao - , Stanford University (Author)
  • Stefan C.B. Mannsfeld - , SLAC National Accelerator Laboratory (Author)
  • Zhenan Bao - , Stanford University (Author)
  • Jianbin Xu - , Chinese University of Hong Kong (Author)
  • Qian Miao - , Chinese University of Hong Kong (Author)

Abstract

A novel self-assembled monolayer (SAM) on AlOy/TiOx is terminated with cyclohexyl groups, an unprecedented terminal group for all kinds of SAMs. The SAM-modified AlOy/TiOx functions as a general dielectric, enabling organic thin-film transistors with a field-effect mobility higher than 5 cm2 V-1 s-1 for both holes and electrons, good air stability with low operating voltage, and general applicability to solution-processed and vacuum-deposited n-type and p-type organic semiconductors.

Details

Original languageEnglish
Pages (from-to)7190-7196
Number of pages7
JournalAdvanced materials
Volume26
Issue number42
Publication statusPublished - 1 Nov 2014
Peer-reviewedYes
Externally publishedYes

External IDs

PubMed 25205623

Keywords

Research priority areas of TU Dresden

ASJC Scopus subject areas

Keywords

  • interface engineering, organic thin-film transistors, self-assembled monolayers (SAMs)

Library keywords