Resonant inelastic x-ray scattering studies of elementary excitations

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Luuk J.P. Ament - , Leiden University (Author)
  • Michel Van Veenendaal - , Argonne National Laboratory, Northern Illinois University (Author)
  • Thomas P. Devereaux - , Stanford Linear Accelerator Center (SLAC) (Author)
  • John P. Hill - , Brookhaven National Laboratory (Author)
  • Jeroen Van Den Brink - , Leibniz Institute for Solid State and Materials Research Dresden (Author)

Abstract

In the past decade, resonant inelastic x-ray scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron x-ray radiation sources and of advanced photon detection instrumentation. The technique's unique capability to probe elementary excitations in complex materials by measuring their energy, momentum, and polarization dependence has brought RIXS to the forefront of experimental photon science. Both the experimental and theoretical RIXS investigations of the past decade are reviewed, focusing on those determining the low-energy charge, spin, orbital, and lattice excitations of solids. The fundamentals of RIXS as an experimental method are presented and then the theoretical state of affairs, its recent developments, and the different (approximate) methods to compute the dynamical RIXS response are reviewed. The last decade's body of experimental RIXS data and its interpretation is surveyed, with an emphasis on RIXS studies of correlated electron systems, especially transition-metal compounds. Finally, the promise that RIXS holds for the near future is discussed, particularly in view of the advent of x-ray laser photon sources.

Details

Original languageEnglish
Pages (from-to)705-767
Number of pages63
JournalREVIEWS OF MODERN PHYSICS
Volume83
Issue number2
Publication statusPublished - 24 Jun 2011
Peer-reviewedYes
Externally publishedYes

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