Reply to the ‘Comment on “Terahertz pump-probe of liquid water at 12.3 THz”’ by A. F. G. van der Meer, PCCP, 2022, 24, D1CP05216K
Research output: Contribution to journal › Review article › Contributed › peer-review
Contributors
Abstract
As outlined in our paper, we developed a model which is able to explain all recorded THz pump-probe data at 12.3 THz in the static water cell as well as in the liquid jet. The model includes an instantaneous temperature-dependent response by an acoustic phonon, an inherent non-linear response of water, and a slower thermal response. The order of magnitude of the non-linear contributions agrees with previous experimental results by us2 and other groups (see ref. 32, 33 and 35 in ref. 1) as well as with simulations2, which predict an enhanced non-linear response of water in the frequency range of the libration.
Details
Original language | English |
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Pages (from-to) | 13413-13415 |
Number of pages | 3 |
Journal | Physical Chemistry Chemical Physics |
Volume | 2022 |
Issue number | 24(21) |
Early online date | 20 May 2022 |
Publication status | Published - 7 Jun 2022 |
Peer-reviewed | Yes |
Externally published | Yes |
External IDs
ORCID | /0000-0002-8120-8553/work/161409568 |
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