Rechargeable Al-ion batteries

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Caixia Li - , Kyoto University (Author)
  • Chun Chao Hou - , Kyoto University (Author)
  • Liyu Chen - , Kyoto University (Author)
  • Stefan Kaskel - , Chair of Inorganic Chemistry I (Author)
  • Qiang Xu - , Kyoto University, Yangzhou University, Southern University of Science and Technology (Author)

Abstract

Aluminum (Al) is the most abundant metal element in earth crust, together with low cost and high safety. Al-ion batteries (AIBs) have been regarded as potential alternatives to lithium-ion batteries (LIBs) in large scale applications and attracted much attention in current days. In this review, recent developments of AIBs including the electrolyte exploration, electrode design and Al protection are summarized. Both aqueous and non-aqueous electrolytes exhibit important benefits for AIBs, especially ionic liquid electrolytes with high stripping/plating efficiency, which are preferentially discussed here. Furthermore, we highlight the design principles and electrochemical mechanism for carbons, metal compounds as well as new-type positive electrode materials for high-performance AIBs. Besides, we focus on the negative electrode protection with suitable coating layers to reduce dendrite formation and improve electrochemical activation of Al negative electrodes. The accessible characterization techniques that promote the development of AIBs are discussed. Finally, prospects and outlooks of AIBs towards theoretical investigations and practical applications are provided.

Details

Original languageEnglish
Article number100049
JournalEnergyChem
Volume3
Issue number2
Publication statusPublished - Mar 2021
Peer-reviewedYes

Keywords

Sustainable Development Goals

Keywords

  • Al protection, Al-ion batteries, Electrode design, Electrolyte exploration