Quantum Fluctuations of Charge Order Induce Phonon Softening in a Superconducting Cuprate

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • H. Y. Huang - , National Synchrotron Radiation Research Center Taiwan (Author)
  • A. Singh - , National Synchrotron Radiation Research Center Taiwan (Author)
  • C. Y. Mou - , National Tsing Hua University (Author)
  • S. Johnston - , University of Tennessee, Knoxville (Author)
  • A. F. Kemper - , North Carolina State University (Author)
  • J. Van Den Brink - , Chair of Solid State Theory, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • P. J. Chen - , City University of Hong Kong (Author)
  • T. K. Lee - , Academia Sinica - Institute of Physics, National Sun Yat-sen University (Author)
  • J. Okamoto - , National Synchrotron Radiation Research Center Taiwan (Author)
  • Y. Y. Chu - , National Synchrotron Radiation Research Center Taiwan (Author)
  • J. H. Li - , National Synchrotron Radiation Research Center Taiwan, National Tsing Hua University (Author)
  • S. Komiya - , Central Research Institute of Electric Power Industry (Author)
  • A. C. Komarek - , Max Planck Institute for Chemical Physics of Solids (Author)
  • A. Fujimori - , National Synchrotron Radiation Research Center Taiwan, Waseda University (Author)
  • C. T. Chen - , National Synchrotron Radiation Research Center Taiwan (Author)
  • D. J. Huang - , National Synchrotron Radiation Research Center Taiwan, National Tsing Hua University (Author)

Abstract

Quantum phase transitions play an important role in shaping the phase diagram of high-temperature cuprate superconductors. These cuprates possess intertwined orders which interact strongly with superconductivity. However, the evidence for the quantum critical point associated with the charge order in the superconducting phase remains elusive. Here, we reveal the short-range charge orders and the spectral signature of the quantum fluctuations in La2-xSrxCuO4 (LSCO) near the optimal doping using high-resolution resonant inelastic x-ray scattering. On performing calculations through a diagrammatic framework, we discover that the charge correlations significantly soften several branches of phonons. These results elucidate the role of charge order in the LSCO compound, providing evidence for quantum critical scaling and discommensurations associated with charge order.

Details

Original languageEnglish
Article number041038
JournalPhysical Review X
Volume11
Issue number4
Publication statusPublished - Dec 2021
Peer-reviewedYes

Keywords

ASJC Scopus subject areas