Nonadiabatic dynamics of ethylene in femtosecond laser pulses

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

Abstract

The dynamics of the ethylene molecule in femtosecond laser pulses is studied as a function of the laser parameters using an ab initio time-dependent approach, called nonadiabatic quantum molecular dynamics. We predict that, by choosing different femtosecond pulses with well-defined excitation frequencies, one can selectively induce either the isomerization process or different fragmentation phenomena.

Details

Original languageEnglish
Article number023422
Number of pages6
JournalPhysical Review A
Volume72
Issue number2
Publication statusPublished - Aug 2005
Peer-reviewedYes

External IDs

WOS 000231564200151
Scopus 27144507515

Keywords

Keywords

  • QUANTUM MOLECULAR-DYNAMICS, AB-INITIO, RESONANCE RAMAN, EXCITATION, FRAGMENTATION, FORMALISM, CLUSTER, STATES