New angles on the border of antiferromagnetism in NiS2 and URu2 Si2

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • P. G. Niklowitz - , Technical University of Munich, Royal Holloway University of London (Author)
  • C. Pfleiderer - , Technical University of Munich (Author)
  • S. Mühlbauer - , Technical University of Munich (Author)
  • P. Böni - , Technical University of Munich (Author)
  • T. Keller - , Max Planck Institute for Solid State Research, Technical University of Munich (Author)
  • P. Link - , Technical University of Munich (Author)
  • J. A. Wilson - , University of Bristol (Author)
  • M. Vojta - , University of Cologne (Author)
  • J. A. Mydosh - , University of Cologne (Author)

Abstract

Following the border of antiferromagnetism (AF) to zero temperature is a promising route to unconventional metallic and superconducting phases. Many interesting examples of antiferromagnetic quantum phase transitions can only be reached by pressure tuning. The range of quantitative experimental probes, which can be realised in a high-pressure environment is limited. However, advances have recently been made in neutron scattering, where elliptically shaped neutron guides now increase the beam intensity directed to mm size sample for high pressure studies. This has been demonstrated on the simple antiferromagnet NiS2. Neutron scattering also allows highly accurate measurements of the lattice constant via the Larmor diffraction technique, which proved extremely useful in studying the high-pressure phase diagram of the itinerant helimagnet MnSi. We now combined Larmor diffraction with conventional diffraction measurements to investigate the pressure-temperature phase diagram of URu2 Si2 up to 20 kbar. URu2 Si2 offers a further spectacular example for the presence of unconventional phases in the vicinity of antiferromagnetism. In this compound, antiferromagnetism is replaced below approximately 5 kbar by the mysterious "hidden order" (HO) and unconventional superconductivity. Our measurements allow the observation of magnetic order and changes in the a- and c-axis lattice constants across the phase transitions in the same experiment. The results contain clear indications of a first-order transition and strong differences between the AF phase and the HO phase in the coupling to the lattice.

Details

Original languageEnglish
Pages (from-to)2955-2960
Number of pages6
JournalPhysica B: Condensed Matter
Volume404
Issue number19
Publication statusPublished - 15 Oct 2009
Peer-reviewedYes
Externally publishedYes

Keywords

Keywords

  • Border of antiferromagnetism, Elliptic neutron guides, Hidden order in URu Si, High pressure, Larmor diffraction