Nature of Magnetic Excitations in the High-Field Phase of α-RuCl3

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • A. N. Ponomaryov - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • L. Zviagina - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • J. Wosnitza - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Physics of High Magnetic Fields, Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • P. Lampen-Kelley - , Oak Ridge National Laboratory, University of Tennessee, Knoxville (Author)
  • A. Banerjee - , Oak Ridge National Laboratory (Author)
  • J. Q. Yan - , Oak Ridge National Laboratory (Author)
  • C. A. Bridges - , Oak Ridge National Laboratory (Author)
  • D. G. Mandrus - , Oak Ridge National Laboratory, University of Tennessee, Knoxville (Author)
  • S. E. Nagler - , Oak Ridge National Laboratory (Author)
  • S. A. Zvyagin - , Helmholtz-Zentrum Dresden-Rossendorf (Author)

Abstract

We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of α-RuCl3, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements were performed in magnetic fields up to 16 T, applied along the [110] and [100] directions. Several ESR modes were detected. Combining our findings with recent inelastic neutron-and Raman-scattering data, we identified most of the observed excitations. Most importantly, we show that the low-temperature ESR response beyond the boundary of the magnetically ordered region is dominated by single-and two-particle processes with magnons as elementary excitations. The peculiarities of the excitation spectrum in the vicinity of the critical field are discussed.

Details

Original languageEnglish
Article number037202
JournalPhysical review letters
Volume125
Issue number3
Publication statusPublished - 17 Jul 2020
Peer-reviewedYes

External IDs

PubMed 32745422

Keywords

ASJC Scopus subject areas