Mass Transfer Performance and Hydrodynamics of a Bubble Column Reactor at Offshore Floating Conditions

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Nasim Heydari - , Université Laval, Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • Faïçal Larachi - , Université Laval (Author)
  • Ragna Kipping - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • Markus Schubert - , Chair of Chemical Process Engineering, Helmholtz-Zentrum Dresden-Rossendorf (Author)

Abstract

Hydrodynamics and mass transfer characteristics are analyzed in a bubble column subjected to simulated ship motions using a hexapod robot with six-degree-of-freedom motions. Wire-mesh sensors have been used for collecting local gas holdup and flow patterns under nonreactive conditions. Additionally, the electrical conductivity of the liquid phase during CO2 uptake was extracted to determine hydroxide ion consumption rates as an indicator of mass transfer. The two-phase flow patterns in the bubble column operating under offshore conditions deviate significantly from the stationary ones due to the buoyancy-driven lateral migration of bubbles. The consumption rates of hydroxide ions during the chemical absorption of CO2 revealed that the amplitude of oscillations imposed on the bubble column is the dominant factor for the mass transfer in moving columns. Contrarily, the effect of the oscillation frequency is negligible, which is attributed to bubble coalescence and bubble flow maldistribution in the bubble column subjected to rotational oscillations. Bubble-free zones are formed in the liquid phase because of the buoyancy effects in the column tilted from the vertical axis, while the frequency of the oscillations does not add any additional effects to the bubble kinematics. The latter is attributed to the low shear rates maintained over the range of frequencies simulating marine swells.

Details

Original languageEnglish
Pages (from-to)12183-12190
Number of pages8
JournalIndustrial and Engineering Chemistry Research
Volume62
Issue number31
Publication statusPublished - 9 Aug 2023
Peer-reviewedYes

External IDs

WOS 001035698400001

Keywords

Sustainable Development Goals

Keywords

  • Gas-liquid flow, Lift forces, Ellipsoidal bubbles, Packed-beds, Drag

Library keywords