Magnetism and the phase diagram of MnSb2O6

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • C. Koo - , Heidelberg University  (Author)
  • J. Werner - , Heidelberg University  (Author)
  • M. Tzschoppe - , Heidelberg University  (Author)
  • M. Abdel-Hafiez - , National University of Science and Technology "MISiS" (Author)
  • P. K. Biswas - , Rutherford Appleton Laboratory (Author)
  • R. Sarkar - , Technische Universität Dresden (Author)
  • H. -H. Klauss - , Technische Universität Dresden (Author)
  • G. V. Raganyan - , Lomonosov Moscow State University (Author)
  • E. A. Ovchenkov - , Lomonosov Moscow State University (Author)
  • A. Yu. Nikulin - , Southern Federal University (Author)
  • A. N. Vasiliev - , South Ural State Univ, South Ural State University, Nanotechnol Educ & Res Ctr (Author)
  • E. A. Zvereva - , South Ural State Univ, South Ural State University, Nanotechnol Educ & Res Ctr (Author)
  • R. Klingeler - , Heidelberg University  (Author)

Abstract

Static and dynamic magnetic properties of P (3) over bar 1m-phase MnSb2O6 have been studied by means of muon-spin relaxation (mu SR), high-frequency electron-spin resonance (HF-ESR), specific heat, and magnetization studies in magnetic fields up to 25 T. The data imply onset of long-range antiferromagnetic order at T-N = 8 K and a spin-flop-like transition at B-SF approximate to 0.7-1T. Below T-N, muon asymmetry exhibits well-defined oscillations indicating a narrow distribution of the local fields. A competing antiferromagnetic phase appearing below T-N2 = 5.3 K is evidenced by a step in the magnetization and a slight kink of the relaxation rate. Above T-N, both mu SR and HF-ESR data suggest short-range spin order. HF-ESR data show that local magnetic fields persist up to at least 12T(N) approximate to 100 K. Analysis of the antiferromagnetic resonance modes and the thermodynamic spin-flop field suggest zero-field splitting of Delta approximate to 18 GHz which implies small but finite magnetic anisotropy.

Details

Original languageEnglish
Article number224416
Number of pages7
JournalPhysical Review B
Volume97
Issue number22
Publication statusPublished - 15 Jun 2018
Peer-reviewedYes

External IDs

Scopus 85048705359

Keywords

Keywords

  • EXCHANGE, ORDER, CO, NI

Library keywords