Magnetism and electronic dynamics in CuCr2-xSnxS4 spinels studied by transferred hyperfine fields at 119Sn and muon spin rotation and relaxation

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Elaheh Sadrollahi - , Chair of Physics of Quantum Materials (Author)
  • Cynthia P. C. Medrano - , Centro Brasileiro de Pesquisas Físicas (Author)
  • Magno A. V. Heringer - , Centro Brasileiro de Pesquisas Físicas (Author)
  • E. M. Baggio Saitovitch - , Centro Brasileiro de Pesquisas Físicas (Author)
  • Lilian Prodan - , Augsburg University, Moldova State University (Author)
  • Vladimir Tsurkan - , Augsburg University, Moldova State University (Author)
  • F. Jochen Litterst - , Technical University of Braunschweig (Author)

Abstract

We investigated magnetization, muon spin rotation and relaxation (µSR), and 119Sn Mössbauer spectroscopy on Sn substituted CuCr2-xSnxS4 (x = 0.03 and 0.08) spinel compounds. The magnetization and µSR results reveal similar additional low-temperature magnetic transitions around 80 K and 40 K as found for the undoped material, indicating a magnetic ground state deviating from a simple collinear ferromagnet. The observed changes in the Mössbauer spectra are less pronounced and are discussed in view of the different positions of the local probes µ+ and 119Sn and their different magnetic coupling to the magnetic Cr lattice. Above 80 K, both µSR and Mössbauer spectra show temperature-dependent inhomogeneous broadening either due to structural or charge disorder and changing spin dynamics that can be related to a precursor magnetic phase above the well-defined static low-temperature phase.

Details

Original languageEnglish
Article number198
JournalThe European physical journal. B, Condensed matter and complex systems
Volume98
Issue number9
Publication statusPublished - Sept 2025
Peer-reviewedYes

External IDs

unpaywall 10.1140/epjb/s10051-025-01046-6
Scopus 105016903933

Keywords