Magnetic-Field Tuning of the Spin Dynamics in the Quasi-2D Van der Waals Antiferromagnet CuCrP2S6
Research output: Contribution to journal › Research article › Contributed › peer-review
Contributors
Abstract
The use of antiferromagnets in magnetoelectronic devices as counterparts of ferromagnets is a new, rapidly developing trend in spintronics that leverages antiferromagnetic (AFM) magnons for transmitting of spin currents. Van der Waals (vdW) antiferromagnets are particularly attractive in this respect as they possess tunable magnetic properties and can be easily integrated into spintronic devices. In this work, electron spin resonance (ESR) spectroscopy is used to assess the potential of the vdW AFM compound CuCrP2S6 for magnonic applications by exploring the magnetic field (H) dependence of the spectrum of magnon excitations below its AFM ordering temperature TN ≈ 30 K and the correlated spin dynamics above TN. ESR reveals prominent ferromagnetic (FM) spin correlations that persist far above TN suggesting an intrinsically 2D character of the spin dynamics in CuCrP2S6. Most interestingly, at T < TN, CuCrP2S6 features two non-degenerate, i.e., distinct in energy AFM magnon modes at H = 0 which can be tuned to the FM type of collective spin excitations with increasing H. These remarkable properties are favorable for the induction and control of unidirectional spin current in CuCrP2S6 and suggest it as a new functional material for magnetoelectronics.
Details
| Original language | English |
|---|---|
| Article number | e11057 |
| Journal | Advanced functional materials |
| Volume | 36 |
| Issue number | 5 |
| Early online date | 26 Aug 2025 |
| Publication status | Published - 15 Jan 2026 |
| Peer-reviewed | Yes |
Keywords
ASJC Scopus subject areas
Keywords
- antiferromagnetism, electron spin resonance, magnetic anisotropy, spin dynamics, spin wave excitation, van der Waals systems