Magnetic-Field Tuning of the Spin Dynamics in the Quasi-2D Van der Waals Antiferromagnet CuCrP2S6

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Joyal John Abraham - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Yaqian Guo - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Yuliia Shemerliuk - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Sebastian Selter - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Saicharan Aswartham - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Kranthi Kumar Bestha - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Laura T. Corredor - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Anja U.B. Wolter - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Olga Kataeva - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Luka Rogić - , University of Zagreb (Author)
  • Noah Somun - , University of Zagreb (Author)
  • Damjan Pelc - , University of Zagreb (Author)
  • Oleg Janson - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Jeroen van den Brink - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Bernd Büchner - , Chair of Experimental Solid State Physics, Clusters of Excellence ctd.qmat: Complexity, Topology and Dynamics in Quantum Matter, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Vladislav Kataev - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Alexey Alfonsov - , Leibniz Institute for Solid State and Materials Research Dresden (Author)

Abstract

The use of antiferromagnets in magnetoelectronic devices as counterparts of ferromagnets is a new, rapidly developing trend in spintronics that leverages antiferromagnetic (AFM) magnons for transmitting of spin currents. Van der Waals (vdW) antiferromagnets are particularly attractive in this respect as they possess tunable magnetic properties and can be easily integrated into spintronic devices. In this work, electron spin resonance (ESR) spectroscopy is used to assess the potential of the vdW AFM compound CuCrP2S6 for magnonic applications by exploring the magnetic field (H) dependence of the spectrum of magnon excitations below its AFM ordering temperature TN ≈ 30 K and the correlated spin dynamics above TN. ESR reveals prominent ferromagnetic (FM) spin correlations that persist far above TN suggesting an intrinsically 2D character of the spin dynamics in CuCrP2S6. Most interestingly, at T < TN, CuCrP2S6 features two non-degenerate, i.e., distinct in energy AFM magnon modes at H = 0 which can be tuned to the FM type of collective spin excitations with increasing H. These remarkable properties are favorable for the induction and control of unidirectional spin current in CuCrP2S6 and suggest it as a new functional material for magnetoelectronics.

Details

Original languageEnglish
Article numbere11057
JournalAdvanced functional materials
Volume36
Issue number5
Early online date26 Aug 2025
Publication statusPublished - 15 Jan 2026
Peer-reviewedYes

Keywords

Keywords

  • antiferromagnetism, electron spin resonance, magnetic anisotropy, spin dynamics, spin wave excitation, van der Waals systems