Magnetic phase diagram and spin Hamiltonian of antiferromagnet Cs2CoI4
Research output: Contribution to journal › Research article › Contributed › peer-review
Abstract
We report comprehensive thermodynamic and neutron scattering measurements on the S=3/2 antiferromagnet Cs2CoI4, a member of the thoroughly studied family of frustrated magnets Cs2MX4 (M=Cu, Co, Ru, X=Br, Cl, I, O). Unlike previously studied members, Cs2CoI4 undergoes a structural phase transition, for which we determine the low-temperature crystallographic structure. The resulting symmetry reduction strongly affects both the magnetic exchange interactions and single-ion anisotropy. Despite the large parameter space, we propose a minimal magnetic Hamiltonian that reasonably captures the observed excitation spectrum, analyzed using extended SU(4) linear spin-wave theory.
Details
| Original language | English |
|---|---|
| Article number | 054420 |
| Journal | Physical review materials |
| Volume | 10 |
| Issue number | 5 |
| Publication status | Published - 1 May 2026 |
| Peer-reviewed | Yes |