Magnetic phase diagram and crystal-field effects in the kagome-lattice antiferromagnet U3Ru4Al12

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • D. I. Gorbunov - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • I. Ishii - , Hiroshima University (Author)
  • T. Nomura - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • M. S. Henriques - , Czech Academy of Sciences (Author)
  • A. V. Andreev - , Czech Academy of Sciences (Author)
  • M. Uhlarz - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • T. Suzuki - , Hiroshima University (Author)
  • S. Zherlitsyn - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • J. Wosnitza - , Chair of Physics of High Magnetic Fields, Helmholtz-Zentrum Dresden-Rossendorf (Author)

Abstract

We report on the magnetic phase diagram of the distorted kagome-lattice antiferromagnet U3Ru4Al12 determined through measurements of magnetic and elastic properties. For field applied along the [100] and [120] axes of the hexagonal crystal structure, we find pronounced anomalies in the magnetization and elastic moduli that signal the existence of unknown magnetic phases. Our crystal-electric-field (CEF) analysis evidences interlevel quadrupolar interactions between the ground-state singlet and the first excited doublet. These interactions lead to a large softening of the shear elastic modulus C44. The large number of phases and pronounced elastic softening suggest that geometric frustrations and CEF effects play an important role in the physical properties of U3Ru4Al12.

Details

Original languageEnglish
Article number054413
JournalPhysical Review B
Volume99
Issue number5
Publication statusPublished - 15 Feb 2019
Peer-reviewedYes