Magnetic frustration, phase competition, and the magnetoelectric effect in NdFe3(BO3)4

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • J. E. Hamann-Borrero - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • S. Partzsch - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • S. Valencia - , Helmholtz Centre Berlin for Materials and Energy (Author)
  • C. Mazzoli - , Polytechnic University of Milan, European Synchrotron Radiation Facility (Author)
  • J. Herrero-Martin - , European Synchrotron Radiation Facility, Institute of Materials Science of Barcelona (ICMAB-CSIC) (Author)
  • R. Feyerherm - , Helmholtz Centre Berlin for Materials and Energy (Author)
  • E. Dudzik - , Helmholtz Centre Berlin for Materials and Energy (Author)
  • C. Hess - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • A. Vasiliev - , Lomonosov Moscow State University (Author)
  • L. Bezmaternykh - , RAS - Kirensky Institute of Physics, Siberian Branch (Author)
  • B. Büchner - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • J. Geck - , Leibniz Institute for Solid State and Materials Research Dresden (Author)

Abstract

We present an element selective resonant magnetic x-ray scattering study of NdFe3(BO3)4 as a function of temperature and applied magnetic field. Our measurements show that the magnetic order of the Nd sublattice is induced by the Fe spin order. When a magnetic field is applied parallel to the hexagonal basal plane, the helicoidal spin order is suppressed and a collinear ordering, where the moments are forced to align in a direction perpendicular to the applied magnetic field, is stabilized. This result excludes a noncollinear spin order as the origin of the magnetically induced electric polarization in this compound. Instead our data imply that magnetic frustration results in a phase competition, which is the origin of the magnetoelectric response.

Details

Original languageEnglish
Article number267202
JournalPhysical review letters
Volume109
Issue number26
Publication statusPublished - 26 Dec 2012
Peer-reviewedYes

External IDs

ORCID /0000-0002-2438-0672/work/158767783

Keywords

ASJC Scopus subject areas