Magnetic, electrical resistivity, heat-capacity, and thermopower anomalies in CeCuAs2

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Kausik Sengupta - , Tata Institute of Fundamental Research (Author)
  • E. V. Sampathkumaran - , Tata Institute of Fundamental Research, The University of Tokyo (Author)
  • T. Nakano - , The University of Tokyo (Author)
  • M. Hedo - , The University of Tokyo (Author)
  • M. Abliz - , The University of Tokyo (Author)
  • N. Fujiwara - , The University of Tokyo (Author)
  • Y. Uwatoko - , The University of Tokyo (Author)
  • S. Rayaprol - , Tata Institute of Fundamental Research (Author)
  • K. Shigetoh - , Hiroshima University (Author)
  • T. Takabatake - , Hiroshima University (Author)
  • Th Doert - , Chair of Inorganic Chemistry II, TUD Dresden University of Technology (Author)
  • J. P.F. Jemetio - , TUD Dresden University of Technology (Author)

Abstract

The results of magnetic susceptibility (χ), electrical resistivity (ρ), heat-capacity (C), and thermopower (S) measurements on CeCuAs 2, forming in the ZrCuSi2-type tetragonal structure, are reported. Our investigations reveal that Ce is trivalent and there is no clear evidence for long range magnetic ordering down to 45 mK. The ρ behavior is notable in the sense that (i) the temperature (T)-coefficient of ρ is negative in the entire range of measurement (45 mK to 300 K) with large values of ρ, while the S behavior is typical of metallic Kondo lattices, and (ii) ρ is proportional to T-0.6 at low temperatures, without any influence on the exponent by the application of a magnetic field, which does not seem to classify this compound into hither-to-known non-Fermi liquid (NFL) systems. In contrast to the logarithmic increase known for NFL systems, C/T measured down to 0.5 K exhibits a fall below 2 K. The observed properties of this compound are unusual among Ce systems.

Details

Original languageEnglish
Article number064406
Pages (from-to)064406-1-064406-5
Number of pages5
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume70(2004)
Issue number6
Publication statusPublished - 5 Aug 2004
Peer-reviewedYes

External IDs

ORCID /0000-0001-7523-9313/work/159171521