Liquid flow texture analysis in trickle bed reactors using high-resolution gamma ray tomography

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Markus Schubert - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Günther Hessel - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Cornelius Zippe - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Rüdiger Lange - , Chair of Chemical Reaction Engineering and Process Plant, TUD Dresden University of Technology (Author)
  • Uwe Hampel - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)

Abstract

Trickle bed reactor performance and safety may suffer from radial and axial liquid maldistribution and thus from non-uniform utilization of the catalyst packing. Therefore, experimental analysis and fluid dynamic simulation of liquid-gas flow in trickle bed reactors is an important topic in chemical engineering. In the present study for the first time a truly high-resolution gamma ray tomography technique was applied to the quantitative analysis of the liquid flow texture in a laboratory cold flow trickle bed reactor of 90 mm diameter. The objective of this study was to present the comparative analysis of the liquid flow dynamics for two different initial liquid distributions and two different types of reactor configurations. Thus, the hydrodynamic behavior of a glass bead packing was compared to a porous Al2O3 catalyst particle packing using inlet flow from a commercial spray nozzle (uniform initial liquid distribution) and inlet flow from a central point source (strongly non-uniform initial liquid distribution), respectively. The column was operated in downflow mode at a gas flow rate of 180 L h-1 and at liquid flow rates of 15 and 25 L h-1.

Details

Original languageEnglish
Pages (from-to)332-340
Number of pages9
JournalChemical engineering journal
Volume140
Issue number1-3
Publication statusPublished - 1 Jul 2008
Peer-reviewedYes

Keywords

Keywords

  • Gamma ray tomography, Liquid distribution, Liquid saturation, Liquid spreading, Multiphase flow, Trickle bed