Large spin-wave energy gap in the bilayer iridate Sr3Ir2O7: Evidence for enhanced dipolar interactions near the Mott metal-insulator transition

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Jungho Kim - , Argonne National Laboratory (Author)
  • A. H. Said - , Argonne National Laboratory (Author)
  • D. Casa - , Argonne National Laboratory (Author)
  • M. H. Upton - , Argonne National Laboratory (Author)
  • T. Gog - , Argonne National Laboratory (Author)
  • M. Daghofer - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • G. Jackeli - , Max Planck Institute for Solid State Research (Author)
  • J. Van Den Brink - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • G. Khaliullin - , Max Planck Institute for Solid State Research (Author)
  • B. J. Kim - , Argonne National Laboratory (Author)

Abstract

Using resonant inelastic x-ray scattering, we observe in the bilayer iridate Sr 3Ir 2O 7, a spin-orbit coupling driven magnetic insulator with a small charge gap, a magnon gap of ∼92meV for both acoustic and optical branches. This exceptionally large magnon gap exceeds the total magnon bandwidth of ∼70meV and implies a marked departure from the Heisenberg model, in stark contrast to the case of the single-layer iridate Sr 2IrO 4. Analyzing the origin of these observations, we find that the giant magnon gap results from bond-directional pseudodipolar interactions that are strongly enhanced near the metal-insulator transition boundary. This suggests that novel magnetism, such as that inspired by the Kitaev model built on the pseudodipolar interactions, may emerge in small charge-gap iridates.

Details

Original languageEnglish
Article number157402
JournalPhysical review letters
Volume109
Issue number15
Publication statusPublished - 10 Oct 2012
Peer-reviewedYes
Externally publishedYes

Keywords

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