Fermi surface chirality induced in a TaSe2 monosheet formed by a Ta/Bi2Se3 interface reaction

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Andrey Polyakov - , Max Planck Institute of Microstructure Physics (Author)
  • Katayoon Mohseni - , Max Planck Institute of Microstructure Physics (Author)
  • Roberto Felici - , National Research Council of Italy (CNR) (Author)
  • Christian Tusche - , Jülich Research Centre, University of Duisburg-Essen (Author)
  • Ying Jun Chen - , Jülich Research Centre, University of Duisburg-Essen (Author)
  • Vitaly Feyer - , Jülich Research Centre, University of Duisburg-Essen (Author)
  • Jochen Geck - , Chair of Physics of Quantum Materials, Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter (Author)
  • Tobias Ritschel - , Chair of Physics of Quantum Materials, Chair of Solid State Physics/Electronic Properties (Author)
  • Arthur Ernst - , Johannes Kepler University Linz (Author)
  • Juan Rubio-Zuazo - , European Synchrotron Radiation Facility (Author)
  • German R. Castro - , European Synchrotron Radiation Facility (Author)
  • Holger L. Meyerheim - , Max Planck Institute of Microstructure Physics (Author)
  • Stuart S.P. Parkin - , Max Planck Institute of Microstructure Physics (Author)

Abstract

Spin-momentum locking in topological insulators and materials with Rashba-type interactions is an extremely attractive feature for novel spintronic devices and is therefore under intense investigation. Significant efforts are underway to identify new material systems with spin-momentum locking, but also to create heterostructures with new spintronic functionalities. In the present study we address both subjects and investigate a van der Waals-type heterostructure consisting of the topological insulator Bi2Se3 and a single Se-Ta-Se triple-layer (TL) of H-type TaSe2 grown by a method which exploits an interface reaction between the adsorbed metal and selenium. We then show, using surface x-ray diffraction, that the symmetry of the TaSe2-like TL is reduced from D3h to C3v resulting from a vertical atomic shift of the tantalum atom. Spin- and momentum-resolved photoemission indicates that, owing to the symmetry lowering, the states at the Fermi surface acquire an in-plane spin component forming a surface contour with a helical Rashba-like spin texture, which is coupled to the Dirac cone of the substrate. Our approach provides a route to realize chiral two-dimensional electron systems via interface engineering in van der Waals epitaxy that do not exist in the corresponding bulk materials.

Details

Original languageEnglish
Article number2472
JournalNature communications
Volume13
Issue number1
Publication statusPublished - Dec 2022
Peer-reviewedYes

External IDs

PubMed 35513364
ORCID /0000-0002-2438-0672/work/158767750