Excitonic quasiparticles in a spin-orbit Mott insulator

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Jungho Kim - , Argonne National Laboratory (Author)
  • M. Daghofer - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • A. H. Said - , Argonne National Laboratory (Author)
  • T. Gog - , Argonne National Laboratory (Author)
  • J. Van Den Brink - , Chair of Solid State Theory, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • G. Khaliullin - , Max Planck Institute for Solid State Research (Author)
  • B. J. Kim - , Max Planck Institute for Solid State Research, Argonne National Laboratory (Author)

Abstract

In condensed matter systems, out of a large number of interacting degrees of freedom emerge weakly coupled quasiparticles (QPs), in terms of which most physical properties are described. The lack of identification of such QPs is a major barrier for understanding myriad exotic properties of correlated electrons, such as unconventional superconductivity and non-Fermi liquid behaviours. Here we report the observation of a composite particle in a quasi-two-dimensional spin-1/2 antiferromagnet Sr2 IrO4 - an exciton dressed with magnons - that propagates with the canonical characteristics of a QP: a finite QP residue and a lifetime longer than the hopping time scale. The dynamics of this charge-neutral excitation mirrors the fundamental process of the analogous one-hole propagation in the background of spins-1/2, and reveals the same intrinsic dynamics that is obscured for a single, charged-hole doped into two-dimensional cuprates.

Details

Original languageEnglish
Article number4453
JournalNature communications
Volume5
Publication statusPublished - 17 Jul 2014
Peer-reviewedYes