Evidence for current-induced phase coexistence in Ca2RuO4 and its influence on magnetic order

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • K. Jenni - (Author)
  • F. Wirth - (Author)
  • K. Dietrich - , University of Cologne (Author)
  • L. Berger - (Author)
  • Y. Sidis - (Author)
  • S. Kunkemöller - (Author)
  • C. P. Grams - (Author)
  • D. I. Khomskii - (Author)
  • J. Hemberger - (Author)
  • M. Braden - (Author)

Abstract

Combining quasistatic and time-resolved transport measurements with X-ray and neutron diffraction experiments we study the non-equilibrium states that arise in pure and in Ti substituted Ca$_2$RuO$_4$ under the application of current densities. Time-resolved studies of the current-induced switching find a slow conductance relaxation that can be identified with heating and a fast one that unambiguously proves an intrinsic mechanism. The current-induced phase transition leads to complex diffraction patterns. Separated Bragg reflections that can be associated with the metallic and insulating phases by their lattice parameters, indicate a real structure with phase coexistence that strongly varies with temperature and current strength. A third contribution with a $c$ lattice constant in between those of metallic and insulating phases appears upon cooling. At low current densities, this additional phase appears below $\sim$100 K and is accompanied by a suppression of the antiferromagnetic order that otherwise can coexist with current carrying states. A possible origin of the intermediate phase is discussed.

Details

Original languageEnglish
Article number085001
JournalPhysical Review Materials
Volume4
Issue number8
Publication statusPublished - 1 Jul 2020
Peer-reviewedYes
Externally publishedYes

External IDs

Scopus 85092188719

Keywords

Keywords

  • cond-mat.str-el

Library keywords