Electronic structure and ultrafast dynamics of FeAs-based superconductors by angle- and time-resolved photoemission spectroscopy

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • I. Avigo - , University of Duisburg-Essen (Author)
  • S. Thirupathaiah - , Indian Institute of Science Bangalore (Author)
  • E. D.L. Rienks - , Chair of Surface Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • L. Rettig - , University of Duisburg-Essen (Author)
  • A. Charnukha - , University of California at San Diego (Author)
  • M. Ligges - , University of Duisburg-Essen (Author)
  • R. Cortes - , Fritz Haber Institute of the Max Planck Society (Author)
  • J. Nayak - , Max Planck Institute for Chemical Physics of Solids (Author)
  • H. S. Jeevan - , Augsburg University (Author)
  • T. Wolf - , Karlsruhe Institute of Technology (Author)
  • Y. Huang - , University of Amsterdam (Author)
  • S. Wurmehl - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • M. I. Sturza - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • P. Gegenwart - , Augsburg University (Author)
  • M. S. Golden - , University of Amsterdam (Author)
  • L. X. Yang - , Kiel University (Author)
  • K. Rossnagel - , Kiel University (Author)
  • M. Bauer - , Kiel University (Author)
  • B. Büchner - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • M. Vojta - , Chair of Theoretical Solid State Physics (Author)
  • M. Wolf - , Fritz Haber Institute of the Max Planck Society (Author)
  • C. Felser - , Max Planck Institute for Chemical Physics of Solids (Author)
  • J. Fink - , Leibniz Institute for Solid State and Materials Research Dresden, TUD Dresden University of Technology, Max Planck Institute for Chemical Physics of Solids (Author)
  • U. Bovensiepen - , University of Duisburg-Essen (Author)

Abstract

In this article, we review our angle- and time-resolved photoemission studies (ARPES and trARPES) on various ferropnictides. In the ARPES studies, we focus first on the band structure as a function of control parameters. We find near optimally “doped” compounds a Lifshitz transition of hole/electron pocket vanishing type. Second, we investigated the inelastic scattering rates as a function of the control parameter. In contrast to the heavily discussed quantum critical scenario, we find no enhancement of the scattering rate near optimally “doping.” Correlation effects which show up by the non-Fermi-liquid behavior of the scattering rates, together with the Lifshitz transition offer a new explanation for the strange normal state properties and suggests an interpolating superconducting state between BCS and BE condensation. Adding femtosecond time resolution to ARPES provides complementary information on electron and lattice dynamics. We report on the response of the chemical potential by a collective periodic variation coupled to coherent optical phonons in combination with incoherent electron and phonon dynamics described by a three temperature heat bath model. We quantify electron phonon coupling in terms of λ 〈ω〉2 and show that the analysis of the electron excess energy relaxation is a robust approach. The spin density wave ordering leads to a pronounced momentum dependent relaxation dynamics. In the vicinity of kf, hot electrons dissipate their energy by electron–phonon coupling with a characteristic time constant of 200 fs. Electrons at the center of the hole pocket exhibit a four time slower relaxation which is explained by spin-dependent dynamics with its smaller relaxation phase space. This finding has implications beyond the material class of Fe-pnictides because it establishes experimental access to spin-dependent dynamics in materials with spin density waves.

Details

Original languageEnglish
Article number1600382
JournalPhysica Status Solidi (B) Basic Research
Volume254
Issue number1
Publication statusPublished - 1 Jan 2017
Peer-reviewedYes

Keywords

Keywords

  • angle-resolved photoemission spectroscopy, Electronic structure, iron-based superconductors