Electronic confinement and ordering instabilities in colossal magnetoresistive bilayer manganites

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • J. Trinckauf - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • T. Hänke - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • V. Zabolotnyy - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • T. Ritschel - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • M. O. Apostu - , Alexandru Ioan Cuza University of Iaşi (Author)
  • R. Suryanarayanan - , Université Paris-Saclay (Author)
  • A. Revcolevschi - , Université Paris-Saclay (Author)
  • K. Koepernik - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • T. K. Kim - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • M. V. Zimmermann - , German Electron Synchrotron (DESY) (Author)
  • S. V. Borisenko - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • M. Knupfer - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • B. Büchner - , Chair of Experimental Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • J. Geck - , Leibniz Institute for Solid State and Materials Research Dresden (Author)

Abstract

We present angle-resolved photoemission studies of (La 1-zPr z) 2-2xSr 1+2xMn 2O 7 with x=0.4 and z=0.1, 0.2, and 0.4 along with density functional theory calculations and x-ray scattering data. Our results show that the bilayer splitting in the ferromagnetic metallic phase of these materials is small, if not completely absent. The charge carriers are therefore confined to a single MnO 2 layer, which in turn results in a strongly nested Fermi surface. In addition to this, the spectral function also displays clear signatures of an electronic ordering instability well below the Fermi level. The increase of the corresponding interaction strength with z and its magnitude of ∼400meV make the coupling to a bare phonon highly unlikely. Instead we conclude that fluctuating order, involving electronic and lattice degrees of freedom, causes the observed renormalization of the spectral features.

Details

Original languageEnglish
Article number016403
JournalPhysical review letters
Volume108
Issue number1
Publication statusPublished - 4 Jan 2012
Peer-reviewedYes

External IDs

ORCID /0000-0002-2438-0672/work/158767785

Keywords

ASJC Scopus subject areas